Sunday, 20 July 2025

Theoretical Insights and Solvatochromic Behavior of 1,3-Benzodioxole Derivatives | Chapter 6 | Current Research Progress in Physical Science Vol. 3

 

The use of spectroscopic techniques, including UV–vis absorption and fluorescence, combined with quantum chemical calculations, allowed us to gain a comprehensive understanding of the (E)-1-(4-hydroxypiperidin-1-yl)-3-(7-methoxybenzo[d][1,3] dioxol-5-yl)prop-2-en-1-one compounds' photophysical properties. The various solute and solvent interactions were investigated using Catalan's and Kamlet's techniques. The compound's excited state dipole moment was estimated using Lippert, Kawski-Chamma-Viallet, Bakhshiev, and \(E_N^T\) solvent polarity parameters. It had been found that the excited state dipole moment was greater than the dipole moment in the ground state. Variations in the solvent's polarity have a direct impact on the distribution of energy in ES. AS and NAS showed a surge in Stokes' shift, which rises with increasing solvent polarity. There could be specific solute-solvent interactions causing this. The redshift results from an effective intermolecular interface with the ES of the polar solvents caused by a significant distinction between the solute's ES and the spreading of GS charge. Further study was conducted to understand further the compound's molecular properties using computational approaches.

 

 

Author(s) Details

K. N. N. Prasad
Department of Physics, BNMIT, Bangalore, 560 070, India.

 

S. Chandrasekhar
Department of Physics, BNMIT, Bangalore, 560 070, India.

 

Please see the book here:- https://doi.org/10.9734/bpi/crpps/v3/1773

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